Help with anxiety

We recently adopted Rhona, a very sweet 1 1/2 y/o G.R. who was neglected. She is a great companion to ou 2 1/2 y/o G.R. Duncan. She has settled in well except for anxiety behaviors; barking at anything, and chewing on objects other than toys such as area rugs, furniture legs, and just yesterday, a window sill. We can crate her, but then she will chew on her tail. The vet suggested Anxitane, a OTC medication which has a synthetic form of green tea (L-Theanine). We both come home for lunch and let the dogs out to run around for an hour or so, then are home again at 4 pm ish. Does anyone have advice?

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